Jeff, you first need to define
what it is you want to do, what's called a "design criteria." As mentioned, you need to share what your goals are (i.e., marina hopping, anchoring out, long range cruising, use of shorepower or alternator only dependency) and then indicate what house bank size you have.
If you want more out of your alternator, going from an internally regulated 80 to an internally regulated 100A won't make much difference. The acceptance of the battery bank will control your charging ability. While Maine Sail and I disagree a bit about this, an externally regulated alternator will give you (somewhat) greater initial input compared to an internally regulated tapering regulator charge. You can't necessarily just slap an external regulator on your existing alternator because usually OEM alternators will end up getting burnt out from external regulation. OEM alternators with internal regulators are just like car alternators, and don't do as much charging for a depleted house bank as is required.
We need more info to begin to be able to help you address your question meaningfully. What are you trying do is clear, we need to know why, other than "more charge", as far as your boat operation. You may be just fine as you are.